AMMRL: DMSO affects 13C-NMR spectrum?

From: Paul Shin <alchemy_at_csun.edu>
Date: Mon, 22 Oct 2007 19:19:57 -0700

Hello all!

Having done most of my work in CDCl3 or D2O, I have observed some
interesting effects by using d6-DMSO! Have any of you an explanation
for why I can acquire lovely standard 13C and DEPT-135 spectra of a
25 mM ibuprofen sample in CDCl3 quite easily (great S/N with few
scans) whereas if d6-DMSO is used, there is literally no analyte
(ibuprofen) signal in either experiment (under identical conditions-
with tuning and matching done for both samples)- not even in the DEPT
135? I do notice a small effect on the 1H-NMR relative sensitivities-
d6-DMSO giving a slightly lower S/N than that in CDCl3, but the
effect in the 13C-NMR is dramatic.

Any ideas and explanations? Viscosity could affect such a change, but
it would/should be more noticeable on 1H and not 13C NMR. We see this
phenomenon with non-hydrogen-bonding capable analytes as well.

Any clues?

Thanks in advance!
Paul

Paul Shin, Ph.D.
Department of Chemistry and Biochemistry, CSUN
California State University
18111 Nordhoff St
Northridge, CA 91330
818-677-6887 phone
818-677-4068 fax
www.csun.edu/chemistry/Facilities.html
Received on Tue Oct 23 2007 - 10:14:15 MST

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